期刊
ORGANIC & BIOMOLECULAR CHEMISTRY
卷 13, 期 24, 页码 6690-6693出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5ob00520e
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资金
- National Natural Science Foundation of China [21302134]
- Natural Science Foundation of Jiangsu [BK20130338]
- Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD)
We report herein a CuX2-mediated halocyclization of gamma,delta-unsaturated amides for the synthesis of functionalized iminolactones and lactams respectively under mild reaction conditions. Mechanism studies indicated that N-attack cyclization was via a radical route while oxycyclization was via a nucleophilic attack on the activated C-C bond.
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