期刊
JOURNAL OF COLLOID AND INTERFACE SCIENCE
卷 338, 期 2, 页码 573-577出版社
ACADEMIC PRESS INC ELSEVIER SCIENCE
DOI: 10.1016/j.jcis.2009.05.001
关键词
Polypyrrole (PPy); Silver (Ag); SiO2; Composites; Catalysis
资金
- National Nature Science Foundation of China [20534040, 20674026]
- 111 project [B06009]
- National Basic Research Program [2007CB936402, 2007CB936403]
Raspberry-like composites were prepared by coating the silver/polypyrrole core/shell composites onto the surface of silica spheres via oxidation polymerization of pyrrole monomer with [Ag(NH3)(2)](+) ions as oxidants. The whole process allowed the absence of stabilizers, which greatly improved the quality of the conducting polymer composites. The morphology of the resulting composites was investigated, which can be described as raspberry-like; also, the structure and composition of the composites were characterized in detail. A possible formation mechanism was proposed. The present synthetic strategy substantially extended the scope of metal/conducting polymer composite synthesis. The raspberry-like composites exhibited excellent catalytic properties in the reduction of methylene blue dye with the reducing agent of sodium borohydride. (C) 2009 Elsevier Inc. All rights reserved.
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