期刊
JOURNAL OF CHEMICAL TECHNOLOGY AND BIOTECHNOLOGY
卷 86, 期 12, 页码 1488-1494出版社
WILEY
DOI: 10.1002/jctb.2656
关键词
catalytic reactors; degradation; heterogeneous catalysis; membranes
类别
资金
- Nature Science Foundations of China [20977117, 20877025]
- Science and Technology Research Programs of Guangdong Province [0711220600311]
- Nature Foundations of GuangDong and GuangXi Province [92510027501000005, 2011GXNSFB018020]
- Foundation of Industry-Education-Academy Cooperation from GuangDong province
- Education Department of Chinese government [2009A090100047, 2010B090486]
- New Process and Technology Project of GuangZhou EPA [2009-03]
- Education Bureau of GuangDong Province [2010-275]
- Scientific Research Foundation of GuangXi University [DD131006]
BACKGROUND: There is growing interest in employing heterogeneous Fenton-like catalysts in slurry to obtain higher activity. However, fine size particles create problems associated with recovery from the treated water. Therefore, it is highly desirable to develop a novel Fenton-like process that not only has high degradation efficiency of organic pollutants, but also allows for easily reusing the catalysts. RESULT: A new reactor was investigated by coupling the heterogeneous Fenton-like oxidation with membrane separation. Results showed that the FeY catalyst could be almost filtrated by a submerged micro-filtration membrane in the reactor to continuously activate H2O2. For a FeY dose of 1 g L-1 and a residence time of 120 min, the degradation efficiency of AO II reached 97%. CONCLUSIONS: In the new reactor, degradation of AO II occurred continuously and efficiently without an additional FeY separation process. The treatment capacity of this FeY catalyst for wastewater containing 100 mg L-1 AO II in the reactor was estimated to be 82 times that of a reactor in which the catalyst could not be reused. The distinguishing technical feature of this reactor was the reuse of the Fenton-like catalyst. (C) 2011 Society of Chemical Industry
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