期刊
JOURNAL OF CHEMICAL PHYSICS
卷 139, 期 3, 页码 -出版社
AMER INST PHYSICS
DOI: 10.1063/1.4813060
关键词
-
资金
- National Research Foundation of South Africa
A formalism for studying the dynamics of quantum systems embedded in classical spin baths is introduced. The theory is based on generalized antisymmetric brackets and predicts the presence of open-path off-diagonal geometric phases in the evolution of the density matrix. The weak coupling limit of the equation can be integrated by standard algorithms and provides a non-Markovian approach to the computer simulation of quantum systems in classical spin environments. It is expected that the theory and numerical schemes presented here have a wide applicability. (C) 2013 AIP Publishing LLC.
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