期刊
JOURNAL OF CHEMICAL PHYSICS
卷 135, 期 16, 页码 -出版社
AMER INST PHYSICS
DOI: 10.1063/1.3656248
关键词
chaos; chemical equilibrium; chemically reactive flow; reaction kinetics theory; spatiotemporal phenomena; turbulence
资金
- Alexander von Humboldt foundation
We report spatiotemporal chaos in the Oregonator model of the Belousov-Zhabotinsky reaction. Spatiotemporal chaos spontaneously develops in a regime, where the underlying local dynamics show stable limit cycle oscillations (diffusion-induced turbulence). We show that spatiotemporal chaos can be suppressed by a unidirectional flow in the system. With increasing flow velocity, we observe a transition scenario from spatiotemporal chaos via a regime of travelling waves to a stationary steady state. At large flow velocities, we recover the known regime of flow distributed oscillations. (C) 2011 American Institute of Physics. [doi: 10.1063/1.3656248]
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