期刊
JOURNAL OF CHEMICAL PHYSICS
卷 131, 期 21, 页码 -出版社
AIP Publishing
DOI: 10.1063/1.3268922
关键词
-
资金
- NNSF China [20533060, 20773114, 20733006, 20873157]
- National Basic Research Program of China [2006CB922004]
- CAS China [KJCX2.YW.H17]
- RGC Hong Kong SAR Government [604508, 604709]
We propose a nonperturbative quantum dissipation theory, in term of hierarchical quantum master equation, which may be used with a great degree of confidence to various dynamics systems in condensed phases. The theoretical development is rooted in an improved semiclassical treatment of Drude bath, beyond the conventional high temperature approximations. It leads to the new theory a simple but important improvement over the conventional stochastic Liouville equation theory, without extra numerical cost. Its broad range of validity and applicability is extensively demonstrated with two-level electron transfer model systems, where the new theory can be considered as the modified Zusman equation. Criterion is also proposed to estimate the performance of the hierarchical quantum master equation. (C) 2009 American Institute of Physics. [doi: 10.1063/1.3268922]
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据