期刊
JOURNAL OF CHEMICAL AND ENGINEERING DATA
卷 59, 期 8, 页码 2547-2550出版社
AMER CHEMICAL SOC
DOI: 10.1021/je500340b
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资金
- Natural Sciences and Engineering Research Council of Canada (NSERC)
- McGill University
- le Fonds Quebecois de la Recherche sur la Nature et les Technologies (FQRNT)
- Canada Research Chair Program (CRC)
- Eugene Ulmer Lamothe Fund (EUL) in the McGill Department of Chemical Engineering
Equilibrium liquid and gas mole fraction measurements were taken at hydrate liquid vapor equilibrium for the N-2 + CO2 + H2O system. Experimental conditions ranged from 275.1 K to 279.2 K and from 2.7 MPa to 14 MPa. Gaseous mole fractions were compared to literature values to validate that equilibrium was reached. The effect of temperature and pressure changes on the solubility of both gas hydrate formers along isotherms is reported. The thermodynamic region associated with a hydrate structure change affected solubility trends.
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