期刊
NATURE PHOTONICS
卷 9, 期 11, 页码 721-+出版社
NATURE PUBLISHING GROUP
DOI: 10.1038/NPHOTON.2015.179
关键词
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资金
- Deutsche Forschungsgemeinschaft Cluster of Excellence 'Munich Centre for Advanced Photonics'
- Fundacio Cellex Barcelona
- Ministerio de Economa y Competitividad through Plan Nacional [FIS2011-30465-C02-01]
- Catalan Agencia de Gestio D'Ajuts Universitaris i de Recerca
- Laserlab-Europe grant [284464]
- SGR
- ICREA Funding Source: Custom
Powerful coherent light with a spectrum spanning the mid-infrared (MIR) spectral range is crucial for a number of applications in natural as well as life sciences, but so far has only been available from large-scale synchrotron sources(1). Here we present a compact apparatus that generates pulses with a sub-two-cycle duration and with an average power of 0.1 W and a spectral coverage of 6.8-16.4 mu m (at -30 dB). The demonstrated source combines, for the first time in this spectral region, a high power, a high repetition rate and phase coherence. The MIR pulses emerge via difference-frequency generation (DFG) driven by the nonlinearly compressed pulses of a Kerr-lens mode-locked ytterbium-doped yttrium-aluminium-garnet (Yb:YAG) thin-disc oscillator. The resultant 100 MHz MIR pulse train is hundreds to thousands of times more powerful than state-of-the-art frequency combs that emit in this range(2-4), and offers a high dynamic range for spectroscopy in the molecular fingerprint region(4-7) and an ideal prerequisite for hyperspectral imaging(8) as well as for the time-domain coherent control of vibrational dynamics(9-11).
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