期刊
JOURNAL OF APPLIED PHYSICS
卷 115, 期 16, 页码 -出版社
AMER INST PHYSICS
DOI: 10.1063/1.4871290
关键词
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资金
- NSF/DOE Partnership in Plasma Science and Technology (NSF) [CBET-0853777]
- NSF/DOE Partnership in Plasma Science and Technology (DOE) [DE-SC0001169]
- NSF Award, EAGER: Exploring plasma mechanism of synthesis of graphene in arc discharge (NSF) [1249213]
- Directorate For Engineering
- Div Of Chem, Bioeng, Env, & Transp Sys [1249213] Funding Source: National Science Foundation
In this paper, a paper-based ultracapacitors were fabricated by the rod-rolling method with the ink of carbon nanomaterials, which were synthesized by arc discharge under various magnetic conditions. Composites of carbon nanostructures, including high-purity single-walled carbon nanotubes (SWCNTs) and graphene flakes were synthesized simultaneously in a magnetically enhanced arc. These two nanostructures have promising electrical properties and synergistic effects in the application of ultracapacitors. Scanning electron microscope, transmission electron microscope, and Raman spectroscopy were employed to characterize the properties of carbon nanostructures and their thin films. The sheet resistance of the SWCNT and composite thin films was also evaluated by four-point probe from room temperature to the cryogenic temperature as low as 90 K. In addition, measurements of cyclic voltammetery and galvanostatic charging/discharging showed the ultracapacitor based on composites possessed a superior specific capacitance of up to 100 F/g, which is around three times higher than the ultracapacitor entirely fabricated with SWCNT. (C) 2014 AIP Publishing LLC.
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