期刊
JOURNAL OF APPLIED PHYSICS
卷 111, 期 12, 页码 -出版社
AIP Publishing
DOI: 10.1063/1.4728229
关键词
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资金
- U.S. Department of Energy
- EERE
- Vehicle Technologies
- Propulsion Materials Program
- Solid State Solar-Thermal Energy Conversion Center (S3TEC), an Energy Frontier Research Center
- US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001299/DE-FG02-09ER46577]
It was recently predicted [D. Parker D. J. Singh, Phys. Rev. B 82, 035204 (2010)], contrary to then-prevalent opinion, that p-type PbSe would be a good thermoelectric material. This prediction was confirmed in Wang et al. [Adv. Mater. 23, 1367 (2011)], and recent experimental work (Zhang et al. Energy Env. Sci. 5, 5246 (2012)] now indicates that n-type PbSe may show good thermoelectric performance. In light of this work, we now re-examine the thermoelectric performance of n-type PbSe with a revised approximation (not available at the time of the original work) which improves band gap accuracy. We now find that n-type PbSe has large thermopowers characteristic of a high performance material, with values as high in magnitude as 250 mu V/K at 1000K and 300 mu V/K at 800 K. We further find that optimal 1000K n-type doping ranges are between 2 x 10(19) cm(-3) and 7 x 10(19) cm(-3), while at 800K, the corresponding range is from 7 x 10(18) to 4 x 10(19) cm(-3). (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4728229]
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