Negative refractive index and acoustic superlens from multiple scattering in single negative metamaterials

Metamaterials, man-made composite media structured on a scale much smaller than a wavelength, offer surprising possibilities for engineering the propagation of waves(1-6). One of the most interesting of these is the ability to achieve superlensing-that is, to focus or image beyond the diffraction limit(7). This originates from the left-handed behaviour-the property of refracting waves negatively-that is typical of negative index metamaterials(8-10). Yet reaching this goal requires the design of 'double negative' metamaterials, which act simultaneously on the permittivity and permeability in electromagnetics(11,12), or on the density and compressibility in acoustics; this generally implies the use of two different kinds of building blocks(13,14) or specific particles presenting multiple overlapping resonances(15-17). Such a requirement limits the applicability of double negative metamaterials, and has, for example, hampered any demonstration of subwavelength focusing using left-handed acoustic metamaterials(18). Here we show that these strict conditions can be largely relaxed by relying on media that consist of only one type of single resonant unit cell. Specifically, we show with a simple yet general semi-analytical model that judiciously breaking the symmetry of a single negative metamaterial is sufficient to turn it into a double negative one. We then demonstrate that this occurs solely because of multiple scattering of waves off the metamaterial resonant elements, a phenomenon often disregarded in these media owing to their subwavelength patterning. We apply our approach to acoustics and verify through numerical simulations that it allows the realization of negative index acoustic metamaterials based on Helmholtz resonators only. Finally, we demonstrate the operation of a negative index acoustic superlens, achieving subwavelength focusing and imaging with spot width and resolution 7 and 3.5 times better than the diffraction limit, respectively. Our findings have profound implications for the physics of metamaterials, highlighting the role of their subwavelength crystalline structure, and hence entering the realm of metamaterial crystals. This widens the scope of possibilities for designing composite media with novel properties in a much simpler way than has been possible so far.