期刊
JOURNAL OF APPLIED PHYSICS
卷 107, 期 1, 页码 -出版社
AMER INST PHYSICS
DOI: 10.1063/1.3275050
关键词
charge injection; multilayers; organic light emitting diodes; organic semiconductors; phosphorescence; thermionic emission; tunnelling; vacancies (crystal); valence bands
资金
- Air Force Office of Scientific Research and Universal Display Corp.
We study electron and hole injection in MoO3 charge generation layers (CGLs) commonly used for establishing balanced injection in multilayer stacked organic light-emitting diodes (SOLEDs). A compound CGL consisting of 100-A degrees-thick MoO3 and Li-doped 4,7-diphenyl-1,10-phenanthroline in a 1:1 molar ratio is demonstrated to have a high electron generation efficiency. Charge injection from the compound CGL is modeled based on a two-step process consisting of tunneling-assisted thermionic emission over an injection barrier of (1.2 +/- 0.2) eV and a trap level due to oxygen vacancies at (0.06 +/- 0.01) eV above the MoO3 valence band edge. Peak external quantum efficiencies (EQEs) of (10.5 +/- 0.2)%, (10.1 +/- 0.2)%, (8.6 +/- 0.2)%, and (8.9 +/- 0.2)% are obtained for tris-(phenylpyridine)iridium-based electrophosphorescent OLEDs with indium tin oxide (ITO) anode/CGL cathode, CGL anode/CGL cathode, CGL anode/Al cathode, and ITO anode/Al cathode contacts, respectively. Based on our analysis, a three-element green emitting electrophosphorescent SOLED is demonstrated with a peak forward-viewing EQE=(24.3 +/- 1.0)% and a power efficiency of (19 +/- 1) lm/W.
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