期刊
JOURNAL OF APPLIED PHYSICS
卷 104, 期 6, 页码 -出版社
AMER INST PHYSICS
DOI: 10.1063/1.2978376
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资金
- Hong Kong Polytechnic University [A-PA8W]
The effect of oxygen vacancy on the dielectric and electromechanical properties in lead titanate zirconate based ferroelectric ceramics is discussed in this paper. The presence of oxygen vacancy forms a defect-dipole inside a perovskite cell. This defect-dipole contributes to the unswitchable polarization and influences the alignment of the ferroelectric dipole in the same cell as well. The latter is due to the displacement of the B-site cation, which contributes to the switchable polarization. It is found that a double hysteresis emerges when the alignment of defect-dipole conforms with the crystal orientation, which is perpendicular to the measured polarization. Moreover, the optimal electromechanical property can be obtained by careful adjustment of c-domain volume fraction and the alignment of defect dipoles. Monte Carlo simulation based on the four-state Potts model is presented. Calculation results are compared with experiments. (c) 2008 American Institute of Physics. [DOI: 10.1063/1.2978376]
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