Obtaining Best Estimates for the Microphysical and Radiative Properties of Tropical Ice Clouds from TWP-ICE In Situ Microphysical Observations

Best estimates of the bulk microphysical and radiative properties (ice water content, visible extinction, effective radius, and total concentration) are derived for three case studies of tropical ice clouds sampled during the Tropical Warm Pool International Cloud Experiment (TWP-ICE). Two case studies are aged cirrus clouds produced by deep convection (the so-called 27/01 and 29/01 cases), and the third (02/02) is a fresh anvil produced by deep convective activity over the Tiwi Islands. Using crystal images obtained by a Cloud Particle Imager (CPI), it is observed that small ice particles (with maximum dimension D < 50-100 mu m) were predominantly quasi spherical, with the degree of nonsphericity increasing rapidly in the 50 < D < 100-mu m range. For D > 100 mu m, the aged cirrus clouds were predominantly characterized by bullet rosettes and aggregates of bullet rosettes, plates, and columns. In contrast, the fresh anvil had more frequent occurrences of plates, columns, aggregates of plates, and occasionally capped columns. The impact of shattering of large ice crystals on probe tips and the overall quality of the TWP-ICE in situ microphysical measurements are assessed. It is suggested that shattering has a relatively small impact on the CPI and cloud droplet probe (CDP) TWP-ICE data and a large impact on the Cloud Aerosol Spectrometer data, as already documented by others. It is also shown that the CPI size distributions must be multiplied by a factor of 4 to match those of the cloud imaging probe (CIP) for maximum dimension larger than 100 mu m (taken as a reference). A technique [named Best Estimate of Area and Density (BEAD)] to minimize errors associated with the density (rho)-D and projected area (A)-D assumptions in bulk microphysics calculation is introduced and applied to the TWP-ICE data. The method makes direct use of the frequency of occurrence of each particle habit as classified from the CPI data and prescribed rho-D and A D relationships from the literature. This approach produces ice water content (IWC) estimates that are virtually unbiased relative to bulk measures obtained from a counter/low spectrometer and impactor (CSI) probe. In contrast, the use of rho-D and A-D relationships for single habits does produce large biases relative to the CSI observations: from -50% for bullet rosettes to +70%-80% for aggregates. The so-called width, length, area, and perimeter (WLAP) technique, which also makes use of individual CPI images, is found to produce positively biased IWCs (by 40% or so), and has a standard deviation of the errors similar to the BEAD technique. The impact of the large variability of the size distributions measured by different probe combinations on the bulk microphysical properties is characterized. The mean fractional differences with respect to the CSI measurements are small for the CPI + CIP, CPI, and CDP + CIP combinations (2.2%, -0.8%, and -1.1%, respectively), with standard deviations of the fractional differences ranging from 7% to 9%. This result provides an independent validation of the CPI scaling factor. The fractional differences produced between the CPI + CP, CPI, and CDP + CIP combinations for extinction, effective radius, and total concentration are 33%, 10%-20%, and 90%, respectively, with relatively small standard deviations of 5%-8%. The fractional difference on total concentration varies greatly over the concentration range though, with values being larger than a factor of 2 for total concentrations smaller than 40 L(-1), but reducing to 10%-20% for concentrations arger than 100 L(-1). Therefore, caution should be exercised when using total concentrations smaller than 60-80 L(-1) as references for radar-lidar retrieval evaluation.