期刊
NANO LETTERS
卷 15, 期 8, 页码 5569-5573出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.5b02188
关键词
Single molecule electronics; cross conjugation; quantum interference; molecular transistors; three terminal devices; electromigration
类别
资金
- Netherlands Organization for Scientific Research (NWO/OCW)
- FOM
- ERC
It is understood that molecular conjugation plays an important role in charge transport through single-molecule junctions. Here, we investigate electron transport through an anthraquinone based single-molecule three-terminal device. With the use of an electric-field induced by a gate electrode, the molecule is reduced resulting into a 10-fold increase in the off-resonant differential conductance. Theoretical calculations link the change in differential conductance to a reduction-induced change in conjugation, thereby lifting destructive interference of transport pathways.
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