期刊
MOLECULES
卷 20, 期 9, 页码 16103-16126出版社
MDPI
DOI: 10.3390/molecules200916103
关键词
cycloaddition reactions; BINOL-derived phosphoric acids; N-triflyl phosphoramides; enantioselective pericyclic reactions
资金
- Deutsche Forschungsgemeinschaft (DFG) [TS 87/15-1, TS 87/17-1]
- Interdisciplinary Center for Molecular Materials (ICMM)
- Erlangen Catalysis Resource Center (ECRC)
- Friedrich-Ebert-Stiftung
Over the last several years there has been a huge increase in the development and applications of new efficient organocatalysts for enantioselective pericyclic reactions, which represent one of the most powerful types of organic transformations. Among these processes are cycloaddition reactions (e.g., [3+2]; formal [3+3]; [4+2]; vinylogous [4+2] and 1,3-dipolar cycloadditions), which belong to the most utilized reactions in organic synthesis of complex nitrogen- and oxygen-containing heterocyclic molecules. This review presents the breakthrough realized in this field using chiral BINOL-derived phosphoric acids and N-triflyl phosphoramide organocatalysts.
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