4.7 Article

Metal loading effects on carbon-supported Pd electrocatalysts

期刊

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
卷 43, 期 37, 页码 17748-17752

出版社

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.ijhydene.2018.07.137

关键词

Palladium; Metal loading; Electrocatalysts; Cyclic voltammetry; Carbon

资金

  1. CNPq [476690/2013-7]
  2. PROPe/UNESP
  3. CAPES

向作者/读者索取更多资源

We report for the first time effects of altering the amount of Pd supported on high-surface area carbon (Pd/C). Cyclic voltammetry in 0.1 M H2SO4 using Pd/C electrocatalysts with distinct metal-to-carbon ratio, Pd black and a Pd wire electrodes reveals unambiguously metal loading effects, such as a decrease in the peak potential for the reduction of palladium oxide (PdO), an increase of the charges of desorption of hydrogen, and formation/ reduction of PdO with the Pd content. Such effects need to be taken into account when designing Pd-based Fuel Cells electrocatalysts. (C) 2018 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.

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