期刊
INORGANIC CHEMISTRY
卷 51, 期 21, 页码 11349-11355出版社
AMER CHEMICAL SOC
DOI: 10.1021/ic300816r
关键词
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资金
- Spanish Ministry of Economy and Competitiveness (MINECO)
- Fondo Social Europeo from the EU
- Spanish MCYT Projects [MAT2010-17571, MAT2011-29020-C02-02]
- Comunidad Autonoma de Madrid [FAMA S2009/MAT-1756]
- Consolider-Ingenio [CSD2006-2001]
Three Ln-based 2D metal organic frameworks with the formula [Ln(3,5-DSB)(Phen)] (Ln = La, Pr, Nd; 3,5-DSB = 3,5-disulfobenzoate; Phen = 1,10-phenathroline) were hydrothermally synthesized. They belong to two 2D structural types, and their nets own a different topologies. The isostructural La and Pr compounds possess a uninodal 5-connected SP 2-periodic net (6,3). The Nd compound has a binodal 3- and 6-connected kgd net. The novel compounds exhibit excellent catalytic activities toward the cyanosilylation reaction under solvent-free conditions.
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