期刊
INORGANIC CHEMISTRY
卷 50, 期 16, 页码 7367-7369出版社
AMER CHEMICAL SOC
DOI: 10.1021/ic201017r
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资金
- NSF [CHE-0714488, DMR-0747587, DMR-0804408]
- Direct For Mathematical & Physical Scien
- Division Of Materials Research [GRANTS:13732250] Funding Source: National Science Foundation
- Division Of Materials Research
- Direct For Mathematical & Physical Scien [0747587] Funding Source: National Science Foundation
The synthesis, structure, and magnetic properties of a ligand-modified Mn-4 dicubane single-molecule magnet (SMM), [Mn-4(Bet)(4)(mdea)(2)(mdeaH)(2)] (BPh4)(4), are presented, where the cationic SMM units are significantly separated from neighboring molecules in the crystal lattice. There are no cocrystallized solvate molecules, making it an ideal candidate for single-crystal magnetization hysteresis and high-frequency electron paramagnetic resonance studies. Increased control over intermolecular interactions in such materials is a crucial factor in the future application of SMMs.
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