期刊
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
卷 57, 期 38, 页码 12766-12773出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.iecr.8b02873
关键词
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资金
- Natural Science Foundation of China [21776322, 21576298, U1663220, 21476271, 21425627]
- Science and Technology Program of Guangzhou [201804010154, 201804020025]
- Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program
Catalytic oxidation is an important removal route of volatile organic compounds (VOCs) pollution. Traditional thermocatalytic oxidation requires either expensive noble metal catalysts or a high reaction temperature, while most photocatalytic oxidation suffers from a low efficiency for the purification of high concentration or refractory VOCs (e.g., aromatic compounds). Herein, we present an efficient visible-light-induced photothermocatalytic VOCs degradation way through constructing the fluorine ions and cheap Ag nanoparticles comodified SrTiO3 catalyst (Ag/F-STO). A photothermocatalytic synergistic effect is demonstrated on Ag/F-STO, providing a higher degradation efficiency than the contribution sum of photocatalytic oxidation and thermocatalytic oxidation. A higher toluene degradation rate constant than state-of-the-art photocatalytic toluene oxidation process and a (>) 95% conversion of benzene, toluene, and xylene mineralization are achieved on Ag/F-STO by photothermocatalysis at 90 degrees C upon visible light irradiation. The results provide a way for robust and economic VOCs removal and corresponding catalyst design.
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