期刊
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
卷 53, 期 27, 页码 10849-10857出版社
AMER CHEMICAL SOC
DOI: 10.1021/ie501287a
关键词
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资金
- National Basic Research Program of China [2014CB239700]
- Natural Science Foundation of China [21336003, 21006063, 21073120]
- China Postdoctoral Science Foundation [2013M541510]
- Science and Technology Commission of Shanghai Municipality [12DZ0502200]
In this study, we report a facile strategy for constructing three-dimensional (3D) crumpled graphene sheets-wrapped nano-Li4Ti5O12 (LTO@GS) composites using a one-pot spray-drying assisted solid-phase reaction method with anatase TiO2 as a starting material. The proportion of graphene oxide (GO) in the LTO@GS composite greatly influences the phase formation and electrochemical performance of the composite. As an anode material for a nonaqueous, hybrid battery-capacitor (Bat Cap) system, the LTO@GS composite exhibits good high-rate capability and long cycle life. The specific capacitance still retains 90% of the initial value after 20 000 cycles, and the Coulombic efficiencies are close to 100%. This can reasonably be attributed to the interesting crumpled graphene-encapsulated structure and extraordinary synergistic effects between the two components.
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