期刊
IEEE TRANSACTIONS ON DIELECTRICS AND ELECTRICAL INSULATION
卷 20, 期 3, 页码 801-813出版社
IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
DOI: 10.1109/TDEI.2013.6518950
关键词
Streamer; partial discharge; phase resolved PD pattern; dielectric fluid; additives; ionization potential; electron affinity; density functional theory; corrosive sulfur
资金
- BAUR Pruf- und Messtechnik GmbH
Partial discharge (PD) characteristics of hexadecane were studied in a needle-plane electrode geometry under AC field with a 20 mu m tip radius tungsten needle. PD experiments were conducted on samples containing known concentrations of aromatic and corrosive sulfur compounds. Partial discharge inception voltage (PDIV), streamer repetition rates, and phase resolved PD (PRPD) patterns were acquired. Ionization potentials (IP) and electron affinities (EA) of hexadecane and the additives were calculated with density functional theory (DFT) and correlated with the PD characteristics. Low IP and negative EA of the additives relative to hexadecane increased the number of positive and negative streamers initiated, except for additives that contained an electron donating group on the aromatic ring. Low IP and positive EA for polyaromatic hydrocarbons (PAH) and corrosive sulfur compounds decreased the number of negative streamers initiated due to large electron capture cross sections. Copper sulfide particulates caused the greatest changes in PD characteristics as a result of its semi-conductive nature.
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