期刊
LANGMUIR
卷 31, 期 49, 页码 13334-13340出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.langmuir.5b02673
关键词
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资金
- FP7 Marie Curie MULTIFLOW Network [PITN-GA-2008-214919]
- ESA/BELSPO-PRODEX
- BELSPO-muMAST [IAP 7/38]
- Fonds de la Recherche Scientifique - FNRS
Freely receding evaporating sessile droplets of perfectly wetting liquids, for which the observed finite contact angles are attributed to evaporation, are studied with a Mach Zehnder interferometer. The experimentally obtained droplet shapes are found to depart, under some conditions, from the classical macroscopic static profile of a sessile droplet. The observed deviations (or the absence thereof) are explained in terms of a Marangoni flow due to evaporation-induced thermal gradients along the liquid air interface. When such a Marangoni effect is strong, the experimental profiles exhibit a maximum of the slope at a certain distance from the contact line. In this case, the axisymmetric flow is directed from the contact line to the apex (along the liquid air interface), hence delivering more liquid to the center of the droplet and making it appear inflated. These findings are quantitatively confirmed by predictions of a lubrication model accounting for the impact of the Marangoni effect on the droplet shape.
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