Physics, Applied

Article Energy & Fuels

Numerical analysis of solar energy storage within a double pipe utilizing nanoparticles for expedition of melting

M. Sheikholeslami

Summary: This study proposes the combination of thermal storage and solar concentrating systems, and suggests the use of new fins and dispersed ZnO nano-powders to improve the low conduction mode of pure paraffin. The numerical procedure has been verified and the simulation results demonstrate the effectiveness of the proposed configurations.

SOLAR ENERGY MATERIALS AND SOLAR CELLS (2022)

Article Nanoscience & Nanotechnology

Ultrabroad Microwave Absorption Ability and Infrared Stealth Property of Nano-Micro CuS@rGO Lightweight Aerogels

Yue Wu, Yue Zhao, Ming Zhou, Shujuan Tan, Reza Peymanfar, Bagher Aslibeiki, Guangbin Ji

Summary: This study synthesized CuS@rGO aerogels and investigated their pore structure, absorption properties, radar cross section, and infrared emissivity by modulating the additive amounts and reduction methods. The results showed that the aerogels exhibited excellent absorption performance in the ultrabroad bandwidth, effectively reduced the radar cross section, and possessed thermal insulation and infrared stealth versatility.

NANO-MICRO LETTERS (2022)

Article Chemistry, Multidisciplinary

Synergy between Palladium Single Atoms and Nanoparticles via Hydrogen Spillover for Enhancing CO2 Photoreduction to CH4

Peigen Liu, Zixiang Huang, Xiaoping Gao, Xun Hong, Junfa Zhu, Gongming Wang, Yuen Wu, Jie Zeng, Xusheng Zheng

Summary: This study demonstrates the synergistic function between single Pd atoms and Pd nanoparticles on graphitic carbon nitride for selective photocatalytic reduction of CO2 into CH4, providing a new perspective for the development of selective photocatalytic CO2 conversion.

ADVANCED MATERIALS (2022)

Article Chemistry, Physical

Fe Single-Atom Catalysts on MOF-5 Derived Carbon for Efficient Oxygen Reduction Reaction in Proton Exchange Membrane Fuel Cells

Xiaoying Xie, Lu Shang, Xuyang Xiong, Run Shi, Tierui Zhang

Summary: The development of Fe single-atom catalysts using MOF-5 as a precursor has led to the creation of highly-porous carbon with an ultrahigh specific surface area, resulting in improved performance in proton exchange membrane fuel cells for the oxygen reduction reaction. The Fe SAC-MOF-5 catalyst demonstrated excellent half-wave potential and peak power density due to the high density of single Fe atoms and increased exposure of active sites on the external surface area of the carbon support.

ADVANCED ENERGY MATERIALS (2022)

Review Chemistry, Multidisciplinary

Oxygen Evolution Reaction in Alkaline Environment: Material Challenges and Solutions

Xiaohong Xie, Lei Du, Litao Yon, Sehkyu Park, Yang Qiu, Joshua Sokolowski, Wei Wang, Yuyan Shao

Summary: This article reviews the active sites for three mainstream non-precious metal catalysts for the oxygen evolution reaction (OER) and discusses the degradation mechanisms and mitigation strategies for these sites. Additionally, it explores the gaps between the research and development of non-precious metal catalysts for the OER and their application in practical devices.

ADVANCED FUNCTIONAL MATERIALS (2022)

Review Chemistry, Multidisciplinary

Recent Progress in External-Stimulus-Responsive 2D Covalent Organic Frameworks

Pengfei She, Yanyan Qin, Xiang Wang, Qichun Zhang

Summary: This review summarizes the recent progress of smart 2D COFs that show reversible changes in conformation, color, and luminescence in response to external stimuli. The responsive mechanisms, design strategies, and applications in chemical sensors and photoelectronic devices are discussed, providing guidelines for designing novel stimulus-responsive 2D COFs for advanced photoelectronic applications.

ADVANCED MATERIALS (2022)

Review Nanoscience & Nanotechnology

Zinc Anode for Mild Aqueous Zinc-Ion Batteries: Challenges, Strategies, and Perspectives

Jinzhang Yang, Bosi Yin, Ying Sun, Hongge Pan, Wenping Sun, Baohua Jia, Siwen Zhang, Tianyi Ma

Summary: The rapid advance of mild aqueous zinc-ion batteries is driving the development of the energy storage system market. However, the issues of Zn anodes, including dendrite growth, hydrogen evolution, and corrosion, severely affect the performance of ZIBs. This review provides a comprehensive overview of existing Zn anode issues, strategies, frontiers, and development trends. Various strategies for constructing stable Zn anodes are summarized and discussed, and future research directions and prospects are proposed.

NANO-MICRO LETTERS (2022)

Article Chemistry, Multidisciplinary

Electronic Structure Engineering of Single-Atom Ru Sites via Co-N4 Sites for Bifunctional pH-Universal Water Splitting

Chengli Rong, Xiangjian Shen, Yuan Wang, Lars Thomsen, Tingwen Zhao, Yibing Li, Xunyu Lu, Rose Amal, Chuan Zhao

Summary: The development of bifunctional water-splitting electrocatalysts that are efficient and stable over a wide range of pH is crucial but challenging. This study reports an atomically dispersed Ru/Co dual-sites catalyst anchored on N-doped carbon (Ru/Co-N-C) for excellent oxygen evolution reaction (OER) and hydrogen evolution reaction (HER) in both acidic and alkaline electrolytes. The catalyst shows superior performance compared to benchmark catalysts Pt/C and RuO2, with low overpotentials and high current densities. Theoretical calculations and experimental results demonstrate that the introduction of Co-N4 sites into Ru/Co-N-C modifies the electronic structure of Ru and enhances the bonding strength with oxygen/hydrogen intermediate species, leading to improved OER and HER performance. Furthermore, the incorporation of Co-N4 sites improves the corrosion-resistance of Ru/Co-N-C during electrolysis. The Ru/Co-N-C catalyst has been successfully applied in a proton exchange membrane water electrolyzer and shows stable operation at a high current density.

ADVANCED MATERIALS (2022)

Article Chemistry, Physical

Design and performance boost of a MOF-functionalized-wood solar evaporator through tuning the hydrogen-bonding interactions

Yi Lu, Deqi Fan, Ziyi Shen, Hao Zhang, Haolan Xu, Xiaofei Yang

Summary: Interfacial solar evaporation technology is a promising solution for freshwater scarcity. The researchers developed a wood-based solar evaporator that achieved high evaporation rate and efficient removal of harmful substances.

NANO ENERGY (2022)

Article Nanoscience & Nanotechnology

A Perspective for Developing Polymer-Based Electromagnetic Interference Shielding Composites

Yali Zhang, Junwei Gu

Summary: The rapid development of aerospace weapons and equipment, wireless base stations, and 5G communication technologies has increased the demands for polymer-based electromagnetic interference (EMI) shielding composites. However, most of these composites fail to combine high performance and multi-functionality. In response, three possible directions for overcoming these limitations have been proposed, including the construction of efficient conductive networks and the optimization of multi-interfaces for lightweight and multifunction compatibility. This research aims to provide a theoretical basis and technical guidance for the preparation and development of polymer-based EMI shielding composites.

NANO-MICRO LETTERS (2022)

Article Chemistry, Multidisciplinary

Highly Active and Durable Single-Atom Tungsten-Doped NiS0.5Se0.5 Nanosheet @ NiS0.5Se0.5 Nanorod Heterostructures for Water Splitting

Yang Wang, Xiaopeng Li, Mengmeng Zhang, Jinfeng Zhang, Zelin Chen, Xuerong Zheng, Zhangliu Tian, Naiqin Zhao, Xiaopeng Han, Karim Zaghib, Yuesheng Wang, Yida Deng, Wenbin Hu

Summary: A highly active and durable single-atom W-doped electrocatalyst for the hydrogen and oxygen evolution reactions has been successfully developed, exhibiting excellent catalytic activity and long-term stability, surpassing commercial precious-metal catalysts and previously reported transition-metal-based compounds.

ADVANCED MATERIALS (2022)

Article Chemistry, Physical

A Universal Additive Strategy to Reshape Electrolyte Solvation Structure toward Reversible Zn Storage

Tian Chen Li, YewVon Lim, Xue Liang Li, Songzhu Luo, Congjian Lin, Daliang Fang, Sunwen Xia, Ye Wang, Hui Ying Yang

Summary: Adding carbonyl-containing organic solvents can enhance the reversibility of zinc-ion batteries and improve their cycling stability and capacity retention.

ADVANCED ENERGY MATERIALS (2022)

Review Optics

Photonics and thermodynamics concepts in radiative cooling

Shanhui Fan, Wei Li

Summary: Radiative cooling is a passive process that utilizes photon heat flow to remove energy and entropy. Recent breakthroughs in nanophotonics have enabled advances in daytime radiative cooling and sparked intense research efforts in this field. Radiative cooling is now emerging as a frontier in renewable energy research, with significant potential for various applications.

NATURE PHOTONICS (2022)

Article Chemistry, Multidisciplinary

Emerging Materials and Designs for Low- and Multi-Band Electromagnetic Wave Absorbers: The Search for Dielectric and Magnetic Synergy?

Junye Cheng, Huibin Zhang, Mingqiang Ning, Hassan Raza, Deqing Zhang, Guangping Zheng, Qingbin Zheng, Renchao Che

Summary: This article reviews the achievements of low- and multi-frequency EMW absorbers, analyzes design strategies, and elaborates on the corresponding electromagnetic response mechanisms. It is of great significance for the new trends and challenges of EMW absorbers.

ADVANCED FUNCTIONAL MATERIALS (2022)

Article Chemistry, Multidisciplinary

Efficient Alkaline Water/Seawater Hydrogen Evolution by a Nanorod-Nanoparticle-Structured Ni-MoN Catalyst with Fast Water-Dissociation Kinetics

Libo Wu, Fanghao Zhang, Shaowei Song, Minghui Ning, Qing Zhu, Jianqing Zhou, Guanhui Gao, Zhaoyang Chen, Qiancheng Zhou, Xinxin Xing, Tian Tong, Yan Yao, Jiming Bao, Luo Yu, Shuo Chen, Zhifeng Ren

Summary: This study demonstrates a heterogeneous Ni-MoN catalyst with outstanding performance for high-current-density water electrolysis. The catalyst, consisting of nanoparticles and nanorods, possesses abundant active sites and a hydrophilic surface that facilitates gas-release and prevents catalyst degradation. Theoretical calculations confirm the synergistic effect of Ni and MoN, as well as the improved water-dissociation kinetics at the Mo sites.

ADVANCED MATERIALS (2022)

Review Chemistry, Physical

Metal/Covalent-Organic Framework Based Cathodes for Metal-Ion Batteries

Lingjun Kong, Ming Liu, Hui Huang, Yunhua Xu, Xian-He Bu

Summary: Metal-organic frameworks (MOFs) and covalent-organic frameworks (COFs) are emerging families of functional materials with immense potential for high-performance electrode materials for metal-ion batteries. Despite their advantages, MOFs/COFs and their derivatives face challenges as cathode materials.

ADVANCED ENERGY MATERIALS (2022)

Review Chemistry, Multidisciplinary

Review on Nanoparticles and Nanostructured Materials: Bioimaging, Biosensing, Drug Delivery, Tissue Engineering, Antimicrobial, and Agro-Food Applications

Vancha Harish, Devesh Tewari, Manish Gaur, Awadh Bihari Yadav, Shiv Swaroop, Mikhael Bechelany, Ahmed Barhoum

Summary: This review explores the potential and applications of nanomaterials in the biomedical and healthcare fields. It discusses various synthesis methods and different types of nanomaterials. Nanomaterials have promising applications in bioimaging, drug delivery, and antimicrobial fields, among others, with significant prospects for future development.

NANOMATERIALS (2022)

Article Chemistry, Physical

Non-iridium-based electrocatalyst for durable acidic oxygen evolution reaction in proton exchange membrane water electrolysis

Zhen-Yu Wu, Feng-Yang Chen, Boyang Lie, Shen-Wei Yu, Y. Zou Finfrock, Debora Motta Meira, Qiang-Qiang Yan, Peng Zhu, Ming-Xi Chen, Tian-Wei Song, Zhouyang Yin, Hai-Wei Liang, Sen Zhang, Guofeng Wang, Haotian Wang

Summary: A nickel-stabilized ruthenium dioxide catalyst (Ni-RuO2) is reported as a promising alternative to iridium for proton exchange membrane water electrolysis, with high activity and durability in acidic oxygen evolution reaction. Density functional theory studies and operando mass spectroscopy analysis confirm the stabilization effect of nickel on the catalyst lattice, improving the durability of the oxygen evolution reaction.

NATURE MATERIALS (2023)

Review Chemistry, Physical

Anode materials for lithium-ion batteries: A review

P. U. Nzereogu, A. D. Omah, F. I. Ezema, E. I. Iwuoha, A. C. Nwanya

Summary: The demand for eco-friendly and portable energy sources in various industries has led to extensive research and innovation in lithium-ion battery (LIB) technology. LIBs have emerged as the most suitable device for storing electrical power in mobile appliances and electric vehicles, thanks to their lightweight, high energy density, small size, long cycle life, and low pollution. This review article discusses recent advancements in LIB anode materials, their advantages and disadvantages, as well as new approaches to overcome their drawbacks.

APPLIED SURFACE SCIENCE ADVANCES (2022)

Article Chemistry, Multidisciplinary

A Dynamic and Self-Adapting Interface Coating for Stable Zn-Metal Anodes

Zhikun Guo, Lishuang Fan, Chenyang Zhao, Aosai Chen, Nannan Liu, Yu Zhang, Naiqing Zhang

Summary: The zinc-ion battery is gaining attention for its safety and environmental benefits, but dendrite formation and dead zinc accumulation can reduce battery life. A self-adaptable PDMS/TiO2-x coating has been developed to address these issues, inhibiting dendrite growth and maintaining stability during cycling. The cells achieved a high coulombic efficiency after 700 cycles, showcasing the effectiveness of the adaptive interface coating.

ADVANCED MATERIALS (2022)