Journal
FARADAY DISCUSSIONS
Volume 171, Issue -, Pages 393-418Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4fd00028e
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Funding
- Max Planck Society
- Nederlandse organisatie voor Wetenschappelijk Onderzoek
- Carlsberg Foundation
- Swedish Research Council
- Swedish Foundation for Strategic Research
- NSF STC award [1231306]
- Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences, Office of Science, US Department of Energy
- Helmholtz Gemeinschaft through the Young Investigator Program
- excellence cluster The Hamburg Center for Ultrafast Imaging - Structure, Dynamics and Control of Matter at the Atomic Scale of the Deutsche Forschungsgemeinschaft
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We give a detailed account of the theoretical analysis and the experimental results of an X-ray-diffraction experiment on quantum-state selected and strongly laser-aligned gasphase ensembles of the prototypical large asymmetric rotor molecule 2,5-diiodobenzonitrile, performed at the Linac Coherent Light Source [Phys. Rev. Lett. 112, 083002 (2014)]. This experiment is the first step toward coherent diffractive imaging of structures and structural dynamics of isolated molecules at atomic resolution, i.e., picometers and femtoseconds, using X-ray free-electron lasers.
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