Journal
FARADAY DISCUSSIONS
Volume 171, Issue -, Pages 57-80Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4fd00037d
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Funding
- Max Planck Society
- Helmholtz Gemeinschaft through the Young Investigator Program
- Carlsberg Foundation
- excellence cluster The Hamburg Centre for Ultrafast Imaging - Structure, Dynamics and Control of Matter at the Atomic Scale of the Deutsche Forschungsgemeinschaft
- Joachim Herz Stiftung
- Helmholtz Virtual Institute Dynamic Pathways in Multidimensional Landscapes
- Nederlandse organisatie voor Wetenschappelijk Onderzoek
- Swedish Research Council
- Swedish Foundation for Strategic Research
- Office of Basic Energy Sciences, US Department of Energy
- Nanoscale photonic imaging [SFB 755]
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This paper gives an account of our progress towards performing femtosecond time-resolved photoelectron diffraction on gas-phase molecules in a pump-probe setup combining optical lasers and an X-ray free-electron laser. We present results of two experiments aimed at measuring photoelectron angular distributions of laser-aligned 1-ethynyl-4-fluorobenzene (C8H5F) and dissociating, laser-aligned 1,4-dibromobenzene (C6H4Br2) molecules and discuss them in the larger context of photoelectron diffraction on gas-phase molecules. We also show how the strong nanosecond laser pulse used for adiabatically laser-aligning the molecules influences the measured electron and ion spectra and angular distributions, and discuss how this may affect the outcome of future time-resolved photoelectron diffraction experiments.
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