Journal
FARADAY DISCUSSIONS
Volume 176, Issue -, Pages 225-232Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4fd00127c
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Funding
- National Basic Research Program of China (973 program) [2014CB239402]
- National Natural Science Foundation of China [20923006, 21003017, 21120102036, 21106015, 91233201]
- Fundamental Research Funds for the Central Universities
- Swedish Energy Agency
- K & A Wallenberg Foundation
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Three new supramolecular assemblies SA1-SA3 with different linkages between the photosensitizer and catalyst have been synthesized for light driven water oxidation. With flexible -CH2-CH2- chains as the linkage, the assembly SA3 displays the best performance for photocatalytic water oxidation compared with the other two assemblies, a turnover number of 34 has been obtained based on the molecular assembly SA3 in a homogeneous system. This type of assembly connected with flexible linkages represents suitable candidates to construct photoanodes for light driven water splitting in dye sensitized photoelectrochemical devices.
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