Journal
FARADAY DISCUSSIONS
Volume 171, Issue -, Pages 41-56Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4fd00031e
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Funding
- DFG via the Cluster of Excellence: Munich Center for Advanced Photonics
- NSFC
- National Basic Research Program of China
- Shanghai Pujiang Program
- Chemical Sciences, Geosciences, and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy
- Kansas NSF EPSCoR First Award program
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The ionization and fragmentation dynamics of iodine molecules (I-2) are traced using very intense (similar to 10(14) W cm(-2)) ultra-short (similar to 60 fs) light pulses with 87 eV photons of the Free-electron LASer at Hamburg (FLASH) in combination with a synchronized femtosecond optical laser. Within a pump-probe scheme the IR pulse initiates a molecular fragmentation and then, after an adjustable time delay, the system is exposed to an intense FEL pulse. This way we follow the creation of highly-charged molecular fragments as a function of time, and probe the dynamics of multi-photon absorption during the transition from a molecule to individual atoms.
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