Journal
ACS NANO
Volume 9, Issue 12, Pages 12174-12181Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsnano.5b05325
Keywords
biosensor; aqueous process; metal oxide semiconductor; conformal; flexible; field-effect transistor
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Funding
- National Science Foundation [ECCS-1202231]
- Office of Naval Research [N000141410648]
- CalBRAIN Neurotechnology Program
- UCLA
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Conformal bioelectronics enable wearable, noninvasive, and health-monitoring platforms. We demonstrate a simple and straightforward method for producing thin, sensitive In2O3-based conformal biosensors based on field-effect transistors using facile solution-based processing. One-step coating via aqueous In2O3 solution resulted in ultrathin (3.5 nm), high-density, uniform films over large areas. Conformal In2O3-based biosensors on ultrathin polyimide films displayed good device performance, low mechanical stress, and highly conformal contact determined using polydimethylsiloxane artificial skin having complex curvilinear surfaces or an artificial eye. Immobilized In2O3 field-effect transistors with self-assembled monolayers of NH2-terminated Mines functioned as pH sensors. Functionalization with glucose oxidase enabled D-glucose detection at physiologically relevant levels. The conformal ultrathin field-effect transistor biosensors developed here offer new opportunities for future wearable human technologies.
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