Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 137, Issue 35, Pages 11238-11241Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.5b06791
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Funding
- University of California Discovery Grant Program [GCP08-128649]
- U.S. National Science Foundation [CHE-1058835]
- program Severo Ochoa
- MRSEC Program of the NSF [DMR 1121053]
- CSIC
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Zeolites are crystalline inorganic solids with microporous structures, having widespread applications in the fields of catalysis, separation, adsorption, microelectronics, and medical diagnosis. A major drawback of zeolites is the mass transfer limitation due to the small size of the micropores (less than 1 nm). Numerous efforts have been dedicated to integrating mesopores with the microporous zeolite structures by using templating and/or destructive approaches. Here we provide a new strategy for hierarchical pore size zeolite synthesis, without using supramolecular or hard templates. The branching epitaxial growth behavior, as a result of aluminum-zoning, contributes to the formation of the hierarchical porous zeolite structures.
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