Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 137, Issue 50, Pages 15672-15675Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.5b11543
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Funding
- National Science Foundation (NSF) [DMR-1437263]
- U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering [DE-SC0008055]
- U.S. Department of Energy (DOE) [DE-SC0008055] Funding Source: U.S. Department of Energy (DOE)
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We have developed an efficient strategy for the production of stable beta-palladium hydride (PdH0.43) nanocrystals with controllable shapes and remarkable stability. The as-synthesized PdH0.43 nanocrystals showed impressive stability in air at room temperature for over 10 months, which has enabled the investigation of their catalytic property for the first time. The prepared PdH0.43 nanocrystals served as highly efficient catalysts in the oxidation of methanol, showing higher activity than their Pd counterparts. These studies opened a door for further exploration of beta-palladium hydride-based nanomaterials as a new class of promising catalytic materials and beyond.
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