Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 137, Issue 12, Pages 4026-4029Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ja512552g
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Funding
- National Natural Science Foundation of China [51229201, 51272229, 51272231, 51402259, 51432001]
- Zhejiang Provincial Natural Science Foundation of China [LR13E020001]
- China Postdoctoral Science Foundation [2014M550319]
- Welch Foundation [AX-1730]
- National Science Foundation of USA [ECCS 1407443]
- Directorate For Engineering
- Div Of Electrical, Commun & Cyber Sys [1407443] Funding Source: National Science Foundation
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Two-photon processing presents a facile means to tailor the properties of materials in three-dimensions. A two-photon responsive metal-organic framework (MOF) has been realized through the incorporation of a photoactive linker into a MOF via a multivariate strategy. The resulting MOF exhibits a significant one-photon and two-photon excited fluorescence change in response to UV light and infrared femtosecond laser, enabling spatial modulation of the fluorescence property of the MOF. It thus demonstrates the capacity of two-photon patterning and imaging inside the crystal, and the formation of three-dimensional two-photon excited fluorescent structure in a high resolution.
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