Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 137, Issue 51, Pages 16203-16208Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.5b10687
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Funding
- Research Grants Council of Hong Kong [CRP C4030-14G]
- Chinese University of Hong Kong (the Faculty Strategic Development Scheme from the Faculty of Science)
- Chinese University of Hong Kong (One-Off Funding for Research from Research Committee)
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We herein report an efficient synthesis of dibenzo[a,m]rubicene, a new member of nonplanar cydopenta-fused polycyclic aromatic hydrocarbon, and its derivatives. It is found that the conformation and molecular packing of dibenzo[a,m]rubicenes in the solid state can be tuned by the substituting groups, and the silyleth-ynylated derivatives of dibenzo[a,m]rubicenes function as p-type organic semiconductors in solution-processed thin film transistors with field effect mobility of up to 1.0 cm(2) V-1 s(-1).
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