Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 137, Issue 43, Pages 13768-13771Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.5b09329
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Funding
- CREST-JST
- Asahi Glass Foundation
- JSPS
- MEXT, IGER Program in Nagoya University
- Grants-in-Aid for Scientific Research [13J07425] Funding Source: KAKEN
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A redox neutral, highly enantioselective coupling between N-arylaminomethanes and N-sulfonyl aldimines was developed by harnessing the efficient catalysis of P-spiro chiral arylaminophosphonium barfate and a transition-metal photosensitizer under visible light irradiation. This mode of synergistic catalysis provides a powerful strategy for controlling the bond-forming processes of reactive radical intermediates.
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