Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 137, Issue 28, Pages 9153-9159Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.5b04856
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Funding
- Swedish Energy Agency
- Knut and Alice Wallenberg Foundation
- Swedish Research Council
- National Natural Science Foundation of China [21120102036, 91233201]
- National Basic Research Program of China (973 program) [2014CB239402]
- China Scholarship Council
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Light driven water splitting was achieved by a tandem dye-sensitized photoelectrochemical cell with two photoactive electrodes. The photoanode is constituted by an organic dye L0 as photosensitizer and a molecular complex Ru1 as water oxidation catalyst on meso-porous TiO2, while the photocathode is constructed with an organic dye P1 as photoabsorber and a molecular complex Col as hydrogen generation catalyst on nanostructured NiO. By combining the photocathode and the photoanode, this tandem DS-PEC cell can split water by visible light under neutral pH conditions without applying any bias.
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