Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 137, Issue 7, Pages 2776-2784Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.5b00786
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Funding
- NSF [CHE-0948222]
- Stanford Graduate Fellowship (The William K. Bowes, Jr. Foundation)
- Eli Lilly and Company
- Stanford Graduate Fellowship
- John Stauffer Memorial Fellowship
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We report the discovery, synthesis, and application of a new class of non-C-2-symmetric phosphoramidite ligands derived from pyroglutamic acid for use in both oxidative and redox-neutral palladium-catalyzed asymmetric allylic alkylations of 1,3-diketones. The resulting chiral products are typically obtained in high yield with good to excellent levels of enantioselectivity.
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