Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 137, Issue 36, Pages 11558-11561Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.5b06278
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Funding
- JSPS [26708028]
- Japanese-Taiwanese Cooperative Program of the Japan Science and Technology Agency (JST)
- Canon Foundation
- Grants-in-Aid for Scientific Research [13F03505, 24104005, 15K05657, 26708028] Funding Source: KAKEN
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Palladium (Pd) films with perpendicularly aligned mesochannels are expected to provide fascinating electrocatalytic properties due to their low diffusion resistance and the full utilization of their large surface area. There have been no studies on such mesoporous metal films, because of the difficulties in controlling both the vertical alignment of the molecular template and the crystal growth in the metallic pore walls. Here we report an effective approach for the synthesis of mesoporous Pd films with mesochannels perpendicularly aligned to the substrate by an elaborated electrochemical deposition. The films show a superior electrocatalytic activity by taking full advantage of the perpendicularly aligned mesochannels.
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