Journal
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
Volume 2012, Issue 8, Pages 1583-1589Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.201101656
Keywords
Natural products; Amino acids; Nitrogen heterocycles; Iron; Cross-coupling; Oxidation
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Funding
- Important National Science & Technology Specific Projects, China [2009ZX09301-14-1]
- National Natural Science Foundation of China (NSFC) [21102107]
- Chinese Postdoctoral Science Foundation [20110491199]
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A simple method has been developed for functionalizing glycine derivatives by iron-catalysed cross-dehydrogenative coupling (CDC) reactions. In particular, N-arylglycine derivatives reacted with alkynes by oxidative CH/CH coupling reactions to provide a series of substituted quinolines starting from commercially inexpensive materials. Moreover, N-arylglycine esters can be oxidatively coupled to ketones by using FeCl3 in the presence of DDQ.
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