Journal
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
Volume 2012, Issue 33, Pages 6503-6507Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.201201093
Keywords
Redox chemistry; Directing groups; Photochemistry; Non-chelation assistance; Electron transfer
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Funding
- Canada Research Chair (Tier 1)
- E. B. Eddy Foundations
- Canada Foundation for Innovation (CFI)
- Natural Sciences and Engineering Research Council (NSERC) of Canada
- Fonds Quebecois de la Recherche sur la Nature et les Technologies (FQRNT) Centre for Green Chemistry and Catalysis
- McGill University
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A RuII photocatalytic method was developed for the direct mono-benzoyloxylation of electron-rich aromatic and heteroaromatic systems even with an excess amount of benzoyl peroxide. The reaction was conducted at room temperature under visible light. The direct ArCH benzoyloxylations occur without the assistance of any directing groups and can also tolerate various functional groups that have already shown diverse reactivities in transition-metal catalysis.
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