Journal
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
Volume 2013, Issue 3, Pages 453-455Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.201201316
Keywords
Natural products; Alkaloids; Biomimetic synthesis; Multicomponent reactions; Amino acids
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The one-step cascade assembly of the central core of halichonadins K and L, two dimeric sesquiterpenoids of marine origin, is described for a model system providing suitable conditions towards the total synthesis of the two molecules. A biomimetic multicomponent reaction involving a glycine, a C-5 unit presumably derived from lysine, and an isocyanide mimic of the terpene decalins is studied.
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