Journal
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
Volume 2012, Issue 29, Pages 5655-5659Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.201200863
Keywords
Organocatalysis; Enamines; Copper; Michael addition; Aldehydes
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Funding
- Korea Research Foundation [2011-0030745, 2011-0005996]
- National Research Foundation of Korea [2009-0094046, 2010-0002396, 과C6A2404] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
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The combination of a copper complex and a chiral amine organocatalyst induces the formation of multifunctionalized aldehydes from aromatic and aliphatic allylic alcohols. Reactions occur with excellent levels of enantioselectivity, under environmentally benign conditions, and without involving stoichiometric amounts of chemical oxidants for the oxidation of the allylic alcohols or rigorous reaction conditions for transition-metal catalysis.
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