Journal
EUROPEAN JOURNAL OF ORGANIC CHEMISTRY
Volume 2008, Issue 7, Pages 1195-1202Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejoc.200700868
Keywords
macrolides; hydrolytic kinetic resolution; sharpless asymmetric dihydroxylation; cross metathesis; ring-closing metathesis
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An efficient total synthesis of decarestrictine D has been achieved using cross-metathesis or ring-closing metathesis and Yamaguchi macrolactonization as key steps. The stereogenic centres were generated by means of hydrolytic kinetic resolution (HKR) and Sharpless asymmetric dihydroxylation (AD).
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