Journal
EUROPEAN JOURNAL OF INORGANIC CHEMISTRY
Volume 2013, Issue 26, Pages 4541-4545Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejic.201300634
Keywords
Carbon dioxide fixation; Homogeneous catalysis; Aluminum; Copolymerization; N,O ligands
Categories
Funding
- Helmholtz Research School
- Bundesministeriums fur Bildung und Forschung (BMBF)- [Forderkennzeichen 01RC0901A]
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The coupling reaction of epoxides and CO2 is in the focus of many research activities in academia as well as in the industry. In this contribution we report on a versatile aluminum-based homogeneous catalyst utilizing an easy-to-synthesize N2O2 ligand system in combination with various cocatalysts, all of them producing pure alternating poly(cyclohexene carbonate)s with M-n values in the range 10000-15000 gmol(-1). This system also efficiently catalyzes the formation of propylene carbonate.
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