Journal
EUROPEAN JOURNAL OF INORGANIC CHEMISTRY
Volume -, Issue 22, Pages 3460-3466Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ejic.200800421
Keywords
rhodium; nanoparticles; catalysis; enantioselectivity; hydroformylation
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Funding
- Spanish Ministerio de Educacion y Ciencia [CTQ2007-62288/BQU]
- Consolider Ingenio [CSD2006-0003]
- Generalilat de Catalunya [2005SGR007777]
- Egide [(PAI 07165RE)]
- CNRS [(PICS 2428 Picasso 04230PL]
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The organometallic synthesis of rhodium nanoparticles stabilized with diphosphite ligands is described. These nanoparticles were investigated as catalysts in the styrene hydroformylation reaction, and their activity and selectivity were compared with those of similar molecular complexes, NMR spectroscopic studies performed during the course of the catalytic reaction showed that the synthesized nanoparticles are not stable and produce molecular species. (C) Wiley-VCH Verlag GmbH & Co. KGaA, 69451 Weinheim, Germany, 2008.
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