4.5 Article Proceedings Paper

Noble gas migration experiment to support the detection of underground nuclear explosions

Journal

JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY
Volume 307, Issue 3, Pages 2603-2610

Publisher

SPRINGER
DOI: 10.1007/s10967-015-4639-7

Keywords

Underground nuclear explosion; Explosion cavity; On-site inspection; Comprehensive Test-Ban Treaty; Noble gas signatures

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A Noble Gas Migration Experiment injected Xe-127, Ar-37, and sulfur hexafluoride into a former underground nuclear explosion shot cavity. These tracer gases were allowed to migrate from the cavity to near-surface and surface sampling locations and were detected in soil gas samples collected using various on-site inspection sampling approaches. Based on this experiment we came to the following conclusions: (1) SF6 was enriched in all of the samples relative to both Ar-37 and Xe-127. (2) There were no significant differences in the Xe-127 to Ar-37 ratio in the samples relative to the ratio injected into the cavity. (3) The migratory behavior of the chemical and radiotracers did not fit typical diffusion modeling scenarios.

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