4.5 Article

A comparative evaluation of water uptake on several mineral dust sources

Journal

ENVIRONMENTAL CHEMISTRY
Volume 7, Issue 2, Pages 162-170

Publisher

CSIRO PUBLISHING
DOI: 10.1071/EN09122

Keywords

heterogeneous atmospheric chemistry; tropospheric particles

Funding

  1. National Science Foundation [ATM0613124]

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Mineral dust aerosol provides a reactive surface in the troposphere. The reactivity of mineral dust depends on the source region as chemical composition and mineralogy of the aerosol affects its interaction with atmospheric gases. Furthermore, the impact of mineral dust aerosol in atmospheric processes and climate is a function of relative humidity. In this study, we have investigated water uptake of complex dust samples. In particular, water uptake as a function of relative humidity has been measured on three different dust sources that have been characterised using a variety of bulk and surface techniques. For these well-characterised dust samples, it is shown that although there are variations in chemical composition and mineralogy, on a per mass basis, water uptake capacities for the three dusts are very similar and are comparable to single component clay samples. These results suggest that the measured uptake of water of these bulk samples is dominated by the clay component.

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