Journal
ENERGY & ENVIRONMENTAL SCIENCE
Volume 7, Issue 12, Pages 4007-4012Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c4ee01904k
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Funding
- UNC EFRC: Center for Solar Fuels, an Energy Frontier Research Center - U.S. Department of Energy Office of Science, Office of Basic Energy Sciences [DE-SC0001011]
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A single Ru(II) polypyridyl carbene complex catalyzes the electrochemical reduction of CO2 in water with added bicarbonate to give syngas H-2+CO mixtures at the cathode and water oxidation to O-2 at the anode. The H-2/CO ratio in the syngas product can be adjusted between 4 : 1 and 1 : 2 by varying the applied potential and solution pH with overall electrolysis energy efficiencies near 50%.
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