Journal
ENERGY & ENVIRONMENTAL SCIENCE
Volume 6, Issue 12, Pages 3559-3564Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ee42226g
Keywords
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Funding
- U.S. Department of Energy as part of the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center
- U.S. DOE, Office of Science, Office of Basic Energy Sciences [DE-SC0001015, DE-AR0000073]
- National Science Foundation [NSF CBET-0930079]
- Welch Foundation [A-1725]
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IAST calculations reveal that sulfonate ammonium salt grafting renders porous polymer networks (PPN-6-SO3NH4) with exceptionally high adsorption selectivity for CO2 over N-2 and CO2 over CH4. Breakthrough experiments confirm the high CO2 adsorption capacity (1.7 mmol g(-1), 75 mg g(-1)) by feeding 15% CO2 balanced with N-2 at 295 K and 1 bar.
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