Journal
ENERGY & ENVIRONMENTAL SCIENCE
Volume 6, Issue 9, Pages 2597-2602Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c3ee40992a
Keywords
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Funding
- Ministry of Science and Technology of China [2009CB22008, 2013CB834505, 2013CB834804]
- National Science Foundation of China [21090343, 91027041, 50973125]
- Solar Energy Initiative of the Knowledge Innovation Program of the Chinese Academy of Sciences
- Bureau for Basic Research of the Chinese Academy of Sciences
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To prepare a water-soluble catalyst for photocatalytic hydrogen (H-2) evolution, a simple hydrophobic precursor of [FeFe]-H(2)ase mimics, Fe2S2(CO)(6), has been successfully assembled on the surface of CdSe QDs using an interface-directed approach in aqueous/organic solution. The resulting photocatalyst shows the highest efficiency known to date for H-2 evolution with a turnover number (TON) of 8781 vs. Fe2S2(CO)(6) and an initial turnover frequency (TOF) of 596 h(-1) under visible light irradiation in water.
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