Journal
ENERGY & ENVIRONMENTAL SCIENCE
Volume 5, Issue 9, Pages 8538-8542Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c2ee22568a
Keywords
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Funding
- 100 Talents Programme of The Chinese Academy of Sciences
- National Program on Key Basic Research Project of China (973 Program) [2012CB215500]
- Foundation for Innovative Research Groups of the National Natural Science Foundation of China [20921002]
- National Natural Science Foundation of China [21101147]
- Jilin Province Science and Technology Development Program [20100102, 20116008]
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A new hybrid nanostructure composed of three-dimensionally ordered macroporous (3DOM) FeF3 and an homogenous coating of poly(3, 4-ethylenedioxythiophene) (PEDOT) is successfully synthesized using polystyrene (PS) colloidal crystals as hard template, and the coating of PEDOT is achieved through a novel in situ polymerization method. The special nanostructure provides a three-dimensional, continuous, and fast electronic and ionic path in the electrode. Surprisingly, the advantageous combination of 3DOM structure and homogenous coating of PEDOT endows the as-prepared hybrid nanostructures with a stable and high reversible discharge capacity up to 210 mA h g(-1) above 2.0 V at room temperature (RT), and a good rate capability of 120 mA h g(-1) at a high current density of 1 A g(-1), which opens up new opportunities in the development of high performance next-generation lithium-ion batteries (LIBs).
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